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Two-dimensional infrared spectroscopy of neat ice Ih

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Phys. Chem. Chem. Phys., 2016, Advance Article
DOI: 10.1039/C5CP07264F, Paper
Liang Shi, J. L. Skinner, Thomas L. C. Jansen
The assignment of the distinct peaks observed in the OH stretch lineshape of ice Ih is controversial. In contrast to a resent experimental interpretation we find that excitonic cross peaks exist between the dominant exciton states. Opposed to common cases the transition dipole directions between these coupled states are uncorrelated.
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